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Extra info for Advances in Chemical Physics, Volume 13
Then, as vibrational levels begin filling, dissociation first appears. During the dissociation phase, the gas cools and becomes denser because of energy absorbed in the reaction. Of the two competing effects on dissociation rate, cooling predominates because of the powerful temperature effect, and dissociation becomes ever slower until it is equally opposed by recombination at equilibrium. This interplay complicates the interpretation of experiments on shock-wave kinetics of actively coupled reactions.
U. u. u. u. 2 ev. 53 A. 18 x lo8 cmlsec. 42 x lo-l'sec. u. In atomic units, the Bohr frequency relation is simply E = w . 1 Fig. 1. In the Heisenberg representation, the wave function is : Y = [lug exp (-iegt) = Is, [exp ( -iegt) 2 - la, exp (-ie,t)]/Z/Z - exp ( -ie,t)l + 1% [exp ( --iegt) + exp ( --is,t)]. 44 WILLIAM LICHTEN The squares of the coefficients of Is, and Is, give the probabilities for the electron to be on center A or B, respectively: PA = sin2$( [ E ~ E&) (2) and P B = cos2 i([&u - &*It), which are just the equations for the well-known quanta1 resonant exchange.
Richardson, J. , and Brinkley, S. , Mechanics of Reaciing Continua. High Speed Aerodynamics and Jet Propulsion, Vol. 11, Sect. F, Princeton Univ. Press, Princeton, 1956. 4. K h h , T. von, Fundamental Equations in Aerothemchemistry. Selecied Combustion Problems, Vol. 11, Butterworths, London, 1956, pp. 167-184. 5. Eschenroeder, A. , Daiber, J. , Golian, T. , in High Temfierature Aspects of Hypersonic Flow, Pergamon Press, Oxford, 1963, Chapter 11. 6. Eschenroeder, A. , Boyer, D. W.. and Hall, J.